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Preparation of Supported Metal Single-Atom Catalysts on Metal Oxides and Hydroxides

Canio Scarfiello 1, 2, 3 Jeremy Audevard 1 Carole Le Berre 1 Katerina Soulantica 2 Philippe Serp 1 Doan Pham Minh 3
1 LCC - Laboratoire de chimie de coordination
2 LPCNO - Laboratoire de physique et chimie des nano-objets
3 RAPSODEE - Centre de recherche d'Albi en génie des procédés des solides divisés, de l'énergie et de l'environnement
Abstract : During the last decade, great attention has been devoted to supported metal single-atom catalysts (SACs), due to the maximal metal utilization and the unique reactivity of such materials. The preparation of high-loading, stable isolated metal atoms with the desired local environments remains the main challenge for the industrial application of SACs. In this chapter, we discuss in detail the most representative methods for the preparation of SACs on oxide and hydroxide supports to give to the reader a complete idea of the different steps of each procedure employed and the final stability of the deposited single atoms. Moreover, we focus our attention on the “bottom-up” methods, which represent a facile and universal route for the direct preparation of SACs on metal oxides and hydroxides.
Keywords : single atoms single-atom catalysts supported metal single atoms metal oxides metal hydroxides catalyst preparation
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Submitted on : Wednesday, February 23, 2022 - 12:26:49 PM
Last modification on : Tuesday, April 19, 2022 - 4:18:01 PM

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Canio Scarfiello, Jeremy Audevard, Carole Le Berre, Katerina Soulantica, Philippe Serp, et al.. Preparation of Supported Metal Single-Atom Catalysts on Metal Oxides and Hydroxides. Philippe Serp; Doan Pham Minh. Supported Metal Single Atom Catalysis, Wiley, 51-99 (Chap. 2), 2022, 9783527348442. ⟨10.1002/9783527830169.ch2⟩. ⟨hal-03585699⟩

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